Bi2Ge2O7 crystalline structure: a new metastable compound discovered in the Bi2O3–GeO2 system

Описание

Тип публикации: статья из журнала

Год издания: 2025

Идентификатор DOI: 10.1007/s11015-025-01942-3

Ключевые слова: Bi2Ge2O7, crystalline structure, Metastable compound, melt crystallization, bismuth germanate

Аннотация: The paper reports on the crystalline structure of a new metastable compound (Bi2Ge2O7) found in the Bi2O3–GeO2 system. This new phase was synthesized from powders by slow cooling of the melt in a platinum container from 1125 °C. The X‑ray diffraction analysis was used to determine the monoclinic lattice parameters of the crystallinПоказать полностьюe structure (a = 14.81691(4) Å, b = 5.28586(1) Å, c = 9.45669(4) Å, β = 124.4766(2) deg., V = 610.560(3) Å3) and space group C2/c. The sample also contains a small admixture of α‑quartz-type GeO2 (up to 2 wt. %), which could not be removed at this stage of research. Scanning electron microscopy and energy dispersive analysis revealed that the synthesized samples consist of Bi2Ge2O7 plates and Bi2Ge2O7+GeO2 mixture, which is formed along the plate boundaries. The ratio of the initial components (32:68 mol. %) is the most optimal, as it allows obtaining the minimum content of impurity phase (GeO2).

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Издание

Журнал: Metallurgist

Выпуск журнала: Т. 69, 2

Номера страниц: 282-290

ISSN журнала: 00260894

Место издания: Москва

Издатель: Springer New York Consultants Bureau

Персоны

  • Bermeshev T.V. (Siberian Federal University)
  • Zaloga A.N. (Siberian Federal University)
  • Solovyov L.A. (Institute of Chemistry and Chemical Technology, Siberian Branch, Russian Academy of Sciences)
  • Bundin M.P. (Siberian Federal University)
  • Samoilo A.S. (Siberian Federal University)
  • Khlystov D.V. (Siberian Federal University)
  • Plotnikov I.S. (Siberian Federal University)
  • Mazurova E.V. (Institute of Chemistry and Chemical Technology, Siberian Branch, Russian Academy of Sciences)
  • Kovaleva A.A. (Siberian Federal University)
  • Yushkova O.V. (Siberian Federal University)
  • Voroshilov D.S. (Siberian Federal University)
  • Bespalov V.M. (Siberian Federal University)

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